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Nitrogen removal performance of municipal reverse osmosis concentrate with low C/N ratio by membrane-aeratedbiofilm reactor

Xiao Quan, Kai Huang, Mei Li, Meichao Lan, Baoan Li

《环境科学与工程前沿（英文）》 2018年 第12卷 第6期 doi: 10.1007/s11783-018-1047-6

摘要：

MABR exhibits excellent TN removal performance for treating ROC with low C/N ratio.

Operating conditions should be properly controlled to achieve optimal TN removal.

Denitrifying bacteria and NOB are proved notably inhibited by high salinity stress.

The TN removal rate remains over 70% when the NaCl addition amount is below 20 g/L.

关键词： Membrane-aerated biofilm reactor (MABR)     Salinity     Total nitrogen     Reverse osmosis concentrate    

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Nitrifying population dynamics in a redox stratified membrane biofilm reactor (RSMBR) for treating ammonium-rich

Rongchang WANG, Xinmin ZHAN, Yalei ZHANG, Jianfu ZHAO

《环境科学与工程前沿（英文）》 2011年 第5卷 第1期   页码 48-56 doi: 10.1007/s11783-011-0305-7

摘要： Nitrogen removal performance and nitrifying population dynamics were investigated in a redox stratified membrane biofilm reactor (RSMBR) under oxygen limited condition to treat ammonium-rich wastewater. When the loading rate increased from 11.1±1.0 to , the nitrogen removal in the RSMBR system increased from 18.0±9.6 mgN·d to 128.9±61.7 mgN·d . Shortcut nitrogen removal was achieved with nitrite accumulation of about . Confocal micrographs showed the stratified distributions of nitrifiers and denitrifiers in the membrane aerated biofilms (MABs) at day 120, i.e., ammonia and nitrite oxidizing bacteria (AOB and NOB) were dominant in the region adjacent to the membrane, while heterotrophic bacteria propagated at the top of the biofilm. Real-time qPCR results showed that the abundance of gene was two orders of magnitude higher than the abundance of gene in the MABs. However, the gene was always detected during the operation time, which indicates the difficulty of complete washout of NOB in MABs. The growth of heterotrophic bacteria compromised the dominance of nitrifiers in biofilm communities, but it enhanced the denitrification performance of the RSMBR system. Applying a high ammonia loading together with oxygen limitation was found to be an effective way to start nitrite accumulation in MABs, but other approaches were needed to sustain or improve the extent of nitritation in nitrogen conversion in MABs.

关键词： ammonium-rich wastewater     membrane biofilm reactor     nitrification     redox stratification     shortcut nitrogen removal    

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Mercury removal from flue gas using nitrate as an electron acceptor in a membrane biofilm reactor

《环境科学与工程前沿（英文）》 2022年 第16卷 第2期 doi: 10.1007/s11783-021-1454-y

摘要：

Membrane bioreactor achieved mercury removal using nitrate as an electron acceptor.

关键词： Mercury removal     Oxygen     Ferrous sulfide     Transformation of mercury     Microbial community    

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Bioreduction of nitrate in groundwater using a pilot-scale hydrogen-based membrane biofilm reactor

Youneng TANG, Michal ZIV-EL, Chen ZHOU, Jung Hun SHIN, Chang Hoon AHN, Bruce E. RITTMANN, Kerry MEYER, Daniel CANDELARIA, David FRIESE, Ryan OVERSTREET, Rick SCOTT,

《环境科学与工程前沿（英文）》 2010年 第4卷 第3期   页码 280-285 doi: 10.1007/s11783-010-0235-9

摘要： A long-term pilot-scale H-based membrane biofilm reactor (MBfR) was tested for removal of nitrate from actual groundwater. A key feature of this second-generation pilot MBfR is that it employed lower cost polyester hollow fibers and still achieved high loading rate. The steady-state maximum nitrate surface loading at which the effluent nitrate and nitrite concentrations were below the Maximum Contaminant Level (MCL) was at least 5.9 g·N·(m·d), which corresponds to a maximum volumetric loading of at least 7.7 kg·N·(m·d) . The steady-state maximum nitrate surface area loading was higher than the highest nitrate surface loading reported in the first-generation MBfRs using composite fibers (2.6 g·N·(m·d)). This work also evaluated the H-utilization efficiency in MBfR. The measured H supply rate was only slightly higher than the stoichiometric H-utilization rate. Thus, H utilization was controlled by diffusion and was close to 100% efficiency, as long as biofilm accumulated on the polyester-fiber surface and the fibers had no leaks.

关键词： denitrification     groundwater treatment     hydrogen     membrane biofilm reactor (MBfR)     polyester fiber    

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Performance of a hybrid anaerobic-contact oxidation biofilm baffled reactor for the treatment of decentralized

Minmin LIU,Ying ZHAO,Beidou XI,Li’an HOU,Xunfeng XIA

《环境科学与工程前沿（英文）》 2014年 第8卷 第4期   页码 598-606 doi: 10.1007/s11783-013-0576-2

摘要： A novel hybrid anaerobic-contact oxidation biofilm baffled reactor (HAOBR) was developed to simultaneously remove nitrogenous and carbonaceous organic pollutants from decentralized molasses wastewater in the study. The study was based on the inoculation of anaerobic granule sludge in anaerobic compartments and the installation of combination filler in aerobic compartments. The performance of reactor system was studied regarding the hydraulic retention time (HRT), microbial characteristics and the gas water ratio (GWR). When the HRT was 24h and the GWR was 20:1, total ammonia and chemical oxygen demand (COD) of the effluent were reduced by 99% and 91.8%, respectively. The reactor performed stably for treating decentralized molasses wastewater. The good performance of the reactor can be attributed to the high resistance of COD and hydraulic shock loads. In addition, the high solid retention time of contact oxidation biofilm contributed to stable performance of the reactor.

关键词： combination filler     contact oxidation biofilm     food wastewater     anaerobic baffled reactor    

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Impact of dissolved oxygen on the production of nitrous oxide in biological aerated filters

Qiang He, Yinying Zhu, Guo Li, Leilei Fan, Hainan Ai, Xiaoliu Huangfu, Hong Li

《环境科学与工程前沿（英文）》 2017年 第11卷 第6期 doi: 10.1007/s11783-017-0964-0

摘要： Polymerase chain reaction-denaturing gradient gel electrophoresis (PCR-DGGE) and microelectrode technology were employed to evaluate the Nitrous oxide (N O) production in biological aerated filters (BAFs) under varied dissolved oxygen (DO) concentrations during treating wastewater under laboratory scale. The average yield of gasous N O showed more than 4-fold increase when the DO levels were reduced from 6.0 to 2.0 mg·L , indicating that low DO may drive N O generation. PCR-DGGE results revealed that were dominant and may be responsible for N O emission from the BAFs system. While at a low DO concentration (2.0 mg·L ), might play a role. When DO concentration was the limiting factor (reduced from 6.0 to 2.0 mg·L ) for nitrification, it reduced NO -N oxidation as well as the total nitrification. The data from this study contribute to explain how N O production changes in response to DO concentration, and may be helpful for reduction of N O through regulation of DO levels.

关键词： Nitrous oxide     Biological aerated filter     Microelectrode     Dissolved oxygen     Biofilm    

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Comparison and modeling of two biofilm processes applied to decentralized wastewater treatment

Guanglei QIU, Yonghui SONG, Peng YUAN, Liancheng XIANG, Jianfeng PENG, Ping ZENG,

《环境科学与工程前沿（英文）》 2009年 第3卷 第4期   页码 412-420 doi: 10.1007/s11783-009-0141-1

摘要： In order to control water pollution in the rapidly urbanizing South China area, biological contact oxidation (BCO) process and biological aerated filter (BAF) process were applied in a pilot-scale experiment for decentralized wastewater treatment. An investigation to find the optimal parameters of the two biofilm systems was conducted on hydraulic loading, organic loading, and aeration rate. The results indicated that the water reuse criteria required a maximum hydraulic and organic loading of 30.0 m/(m·d) and 4.0 kg COD/(m·d), respectively, as well as a minimum effluent DO of 4.0 mg/L. The utilization of a new media allowed BAF to perform better than BCO. The kinetic description of the COD removal process for BAF and BCO are Yang ZHANG,Zifu LI,Ibrahim B MAHMOOD. [J]. Front. Environ. Sci. Eng., 2014, 8(6): 825-834.Daijun ZHANG, Cui BAI, Ting TANG, Qing YANG. [J]. Front Envir Sci Eng Chin, 2011, 5(2): 291-297.Deming ZHAO, Jie CHENG, Michael R. HOFFMANN. [J]. Front Envir Sci Eng Chin, 2011, 5(1): 57-64.Bo WANG, Wei WAN, Jianlong WANG, . [J]. Front.Environ.Sci.Eng., 2009, 3(4): 380-386. Junxiong LIN , Lan WANG , . [J]. Front.Environ.Sci.Eng., 2009, 3(3): 320-324.Lu LI, Shuguang XIE, Hui ZHANG, Donghui WEN. [J]. Front Envir Sci Eng Chin, 2009, 3(1): 38-47.

关键词： biological contact oxidation     biological aerated filter     decentralized wastewater treatment     kinetic model    

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Effects of carrier-attached biofilm on oxygen transfer efficiency in a moving bed biofilm reactor

Yanling WEI,Xunfei YIN,Lu QI,Hongchen WANG,Yiwei GONG,Yaqian LUO

《环境科学与工程前沿（英文）》 2016年 第10卷 第3期   页码 569-577 doi: 10.1007/s11783-015-0822-x

摘要： Three laboratory-scale moving bed biofilm reactors (MBBR) with different carrier filling ratios ranging from 40% to 60% were used to study the effects of carrier-attached biofilm on oxygen transfer efficiency. In this study, we evaluated the performance of three MBBRs in degrading chemical oxygen demand and ammonia. The three reactors removed more than 95% of -N at an air flow-rate of 60 L·h . The standard oxygen transfer efficiency (αSOTE) of the three reactors was also investigated at air flow-rates ranging from 60 to 100 L·h . These results were compared to αSOTE of wastewater with a clean carrier (no biofilm attached). Results showed that under these process conditions, αSOTE decreased by approximately 70% as compared to αSOTE of wastewater at a different carrier-filling ratio. This indicated that the biofilm attached to the carrier had a negative effect on αSOTE. Mechanism analysis showed that the main inhibiting effects were related to biofilm flocculants and soluble microbial product (SMP). Biofilm flocs could decrease αSOTE by about 20%, and SMP could decrease αSOTE by 30%–50%.

关键词： carrier     biofilm     oxygen transfer efficiency     moving bed biofilm reactor    

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Investigate of in situ sludge reduction in sequencing batch biofilm reactor: Performances, mechanisms

Yonglei Wang, Baozhen Liu, Kefeng Zhang, Yongjian Liu, Xuexin Xu, Junqi Jia

《环境科学与工程前沿（英文）》 2018年 第12卷 第5期 doi: 10.1007/s11783-018-1077-0

摘要：

Microbial metabolism uncoupling, sludge decay is the main mechanism to promote in situ sludge reduction on this biofilm system.

The main reduction mechanism inside the biofilm is sludge decay in the longitudinal distribution of biofilm.

Mizugakiibacter and Azospira anaerobic fermentation bacterium dominate the FSC organisms indicating the dominant mechanism on the biofilm is sludge decay.

The floating spherical carriers with compound of the polyurethane and two fiber balls can effectively blocking suspended sludge, improving Biofilm formation efficiency significantly.

关键词： In situ sludge reduction     Biofilm     Composite floating spherical carriers     Microbial community     SBBR    

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Removal of tetrachlorobisphenol A and the effects on bacterial communities in a hybrid sequencing biofilmbatch reactor-constructed wetland system

Xiaohui Wang, Shuai Du, Tao Ya, Zhiqiang Shen, Jing Dong, Xiaobiao Zhu

《环境科学与工程前沿（英文）》 2019年 第13卷 第1期 doi: 10.1007/s11783-019-1097-4

摘要：

SBBR-CW system was proposed to effectively treat wastewater containing TCBPA.

CW unit contributed more than SBBR to the removal of TCBPA.

TCBPA changed the composition and structure of bacterial community in the system.

GAOs massively grew in SBBR, but did not deteriorate TP removal efficiency.

关键词： SBBR     Constructed wetland     Tetrachlorobisphenol A     Microbial community structure    

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Comparative experiment on treating digested piggery wastewater with a biofilm MBR and conventional MBR

Xiaoyan Song,Rui Liu,Lujun Chen,Tomoki Kawagishi

《环境科学与工程前沿（英文）》 2017年 第11卷 第2期 doi: 10.1007/s11783-017-0919-5

摘要： The BF-MBR displayed higher removal rates of nitrogen, phosphorous and antibiotics. The BF-MBR saved alkali consumption. The removal of antibiotics was influenced significantly by HRT. Membrane filtration greatly contributed to antibiotics removal. A biofilm membrane bioreactor (BF-MBR) and a conventional membrane bioreactor (MBR) were parallelly operated for treating digested piggery wastewater. The removal performance of COD, TN, NH -N, TP as well as antibiotics were simultaneously studied when the hydraulic retention time (HRT) was gradually shortened from 9 d to 1 d and when the ratio of influent COD to TN was changed. The results showed that the effluent quality in both reactors was poor and unstable at an influent COD/TN ratio of 1.0±0.2. The effluent quality was significantly improved as the influent COD/TN ratio was increased to 2.3±0.5. The averaged removal rates of COD, NH -N, TN and TP were 92.1%, 97.1%, 35.6% and 54.2%, respectively, in the BF-MBR, significantly higher than the corresponding values of 91.7%, 90.9%, 17.4% and 31.9% in the MBR. Analysis of 11 typical veterinary antibiotics (from the tetracycline, sulfonamide, quinolone, and macrolide families) revealed that the BF-MBR removed more antibiotics than the MBR. Although the antibiotics removal decreased with a shortened HRT, high antibiotics removals of 86.8%, 80.2% and 45.3% were observed in the BF-MBR at HRT of 5–4 d, 3–2 d and 1 d, respectively, while the corresponding values were only 83.8%, 57.0% and 25.5% in the MBR. Moreover, the BF-MBR showed a 15% higher retention rate of antibiotics and consumed 40% less alkalinity than the MBR. Results above suggest that the BF-MBR was more suitable for digested piggery wastewater treatment.

关键词： Alkalinity     Antibiotics     Biofilm     Digested piggery wastewater (DPW)     Membrane bioreactor    

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methane recovery and exoelectrogen-methanogen evolution from low-strength wastewater in an up-flow biofilmreactor with conductive granular graphite fillers

Zechong Guo, Lei Gao, Ling Wang, Wenzong Liu, Aijie Wang

《环境科学与工程前沿（英文）》 2018年 第12卷 第4期 doi: 10.1007/s11783-018-1074-3

摘要：

Methane yield increased 22 times from low-strength wastewater by applying conductive fillers.

Conductive fillers accelerated the start-up stage of anaerobic biofilm reactor.

Conductive fillers altered methanogens structure.

关键词： Low-strength wastewater     Methane production     Conductive filler     Microbial community structure    

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Comparative study on microbial community in intermittently aerated sequencing batch reactors (SBR) and

Xiaolin Sheng, Rui Liu, Xiaoyan Song, Lujun Chen, Kawagishi Tomoki

《环境科学与工程前沿（英文）》 2017年 第11卷 第3期 doi: 10.1007/s11783-017-0929-3

摘要： A traditional sequencing batch reactor (SBR) and two intermittently aerated sequencing batch reactors (IASBRs) were parallelly operated for treating digested piggery wastewater. Their microbial communities were analyzed, and the nitrogen removal performance was compared during the long–term run. IASBRs demonstrated higher removal rates of total nitrogen (TN) and ammonium nitrogen (NH -N) than the SBR, and also demonstrated higher resistance against TN shock load. It was found that the more switch times between aerobic/anoxic in an IASBR, the higher the removal rates of TN and NH –N. All the reactors were predominated by , and , which were considered to be species of denitrifiers, ammonium oxidizing bacteria (AOB) and nitrite oxidizing bacteria (NOB), respectively. However, the abundance and diversity was of great difference. Compared with SBR, IASBRs achieved higher abundance of denitrification–related bacteria. IASBR 1 with four aerobic/anoxic switch times was detected with 25.63% of , higher than that in IASBR 2 with two aerobic/anoxic switch times (11.57% of ), and much higher than that in the SBR (only 6.19% of ). IASBR 2 had the highest percentage of AOB, while IASBR 1 had the lowest percentage. The denitrifiers abundance was significantly positive correlated with the TN removal rate. However, the NH –N removal rate showed no significant correlation with the AOB abundance, but might relate to the AOB activity which was influenced by the average free ammonium (FA) concentration. was the only NOB genus detectable in all reactors, and were less than 0.03%.

关键词： Digested piggery wastewater     Intermittent aeration     Microbial community     Partial nitrification–denitrification process     Sequencing batch reactor (SBR)    

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Interlayer-confined two-dimensional manganese oxide-carbon nanotube catalytic ozonation membrane for

《化学科学与工程前沿（英文）》 2022年 第16卷 第5期   页码 731-744 doi: 10.1007/s11705-021-2110-6

摘要： Catalytic ozonation technology has attracted copious attention in water purification owing to its favorable oxidative degradation of pollutants and mitigation of membrane fouling capacity. However, its extensive industrial application has been restricted by the low ozone utilization and limited mass transfer of the short-lived radical species. Interlayer space-confined catalysis has been theoretically proven to be a viable strategy for achieving high catalytic efficiency. Here, a two-dimensional MnO2-incorporated ceramic membrane with tunable interspacing, which was obtained via the intercalation of a carbon nanotube, was designed as a catalytic ozonation membrane reactor for degrading methylene blue. Benefiting from the abundant catalytic active sites on the surface of two-dimensional MnO2 as well as the ultralow mass transfer resistance of fluids due to the nanolayer confinement, an excellent mineralization effect, i.e., 1.2 mg O3(aq) mg–1 TOC removal (a total organic carbon removal rate of 71.5%), was achieved within a hydraulic retention time of 0.045 s of pollutant degradation. Further, the effects of hydraulic retention time and interlayer spacing on methylene blue removal were investigated. Moreover, the mechanism of the catalytic ozonation employing catalytic ozonation membrane was proposed based on the contribution of the Mn(III/IV) redox pair to electron transfer to generate the reactive oxygen species. This innovative two-dimensional confinement catalytic ozonation membrane could act as a nanoreactor and separator to efficiently oxidize organic pollutants and enhance the control of membrane fouling during water purification.

关键词： catalytic membrane reactor     catalytic ozonation     nanoconfinement     two-dimensional manganese oxide    

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Isolation and application of an ibuprofen-degrading bacterium to a biological aerated filter for the

Bingjie Xu, Gang Xue, Xing Yang

《环境科学与工程前沿（英文）》 2018年 第12卷 第5期 doi: 10.1007/s11783-018-1080-5

摘要：

• An ibuprofen-degrading strain, Serratia marcescens BL1, was isolated and identified.

• The effects of various factors on ibuprofen degradation by BL1 were evaluated.

• Strain BL1 was applied to a laboratory-scale biological aerated filter system.

• Strain BL1 was stable in both static tests and in the biological aerated filter system.

关键词： Ibuprofen     Biological aerated filter     Degrading bacterium     Serratia marcescens    

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标题 作者 时间 类型 操作

Nitrogen removal performance of municipal reverse osmosis concentrate with low C/N ratio by membrane-aeratedbiofilm reactor

Xiao Quan, Kai Huang, Mei Li, Meichao Lan, Baoan Li

期刊论文

Nitrifying population dynamics in a redox stratified membrane biofilm reactor (RSMBR) for treating ammonium-rich

Rongchang WANG, Xinmin ZHAN, Yalei ZHANG, Jianfu ZHAO

期刊论文

Mercury removal from flue gas using nitrate as an electron acceptor in a membrane biofilm reactor

期刊论文

Bioreduction of nitrate in groundwater using a pilot-scale hydrogen-based membrane biofilm reactor

Youneng TANG, Michal ZIV-EL, Chen ZHOU, Jung Hun SHIN, Chang Hoon AHN, Bruce E. RITTMANN, Kerry MEYER, Daniel CANDELARIA, David FRIESE, Ryan OVERSTREET, Rick SCOTT,

期刊论文

Performance of a hybrid anaerobic-contact oxidation biofilm baffled reactor for the treatment of decentralized

Minmin LIU,Ying ZHAO,Beidou XI,Li’an HOU,Xunfeng XIA

期刊论文

Impact of dissolved oxygen on the production of nitrous oxide in biological aerated filters

Qiang He, Yinying Zhu, Guo Li, Leilei Fan, Hainan Ai, Xiaoliu Huangfu, Hong Li

期刊论文

Comparison and modeling of two biofilm processes applied to decentralized wastewater treatment

Guanglei QIU, Yonghui SONG, Peng YUAN, Liancheng XIANG, Jianfeng PENG, Ping ZENG,

期刊论文

Effects of carrier-attached biofilm on oxygen transfer efficiency in a moving bed biofilm reactor

Yanling WEI,Xunfei YIN,Lu QI,Hongchen WANG,Yiwei GONG,Yaqian LUO

期刊论文

Investigate of in situ sludge reduction in sequencing batch biofilm reactor: Performances, mechanisms

Yonglei Wang, Baozhen Liu, Kefeng Zhang, Yongjian Liu, Xuexin Xu, Junqi Jia

期刊论文

Removal of tetrachlorobisphenol A and the effects on bacterial communities in a hybrid sequencing biofilmbatch reactor-constructed wetland system

Xiaohui Wang, Shuai Du, Tao Ya, Zhiqiang Shen, Jing Dong, Xiaobiao Zhu

期刊论文

Comparative experiment on treating digested piggery wastewater with a biofilm MBR and conventional MBR

Xiaoyan Song,Rui Liu,Lujun Chen,Tomoki Kawagishi

期刊论文

methane recovery and exoelectrogen-methanogen evolution from low-strength wastewater in an up-flow biofilmreactor with conductive granular graphite fillers

Zechong Guo, Lei Gao, Ling Wang, Wenzong Liu, Aijie Wang

期刊论文

Comparative study on microbial community in intermittently aerated sequencing batch reactors (SBR) and

Xiaolin Sheng, Rui Liu, Xiaoyan Song, Lujun Chen, Kawagishi Tomoki

期刊论文

Interlayer-confined two-dimensional manganese oxide-carbon nanotube catalytic ozonation membrane for

期刊论文

Isolation and application of an ibuprofen-degrading bacterium to a biological aerated filter for the

Bingjie Xu, Gang Xue, Xing Yang

期刊论文